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Abstract
A coupled heat and mass transfer model is developed for batch #uidized-bed drying of moist porous particles considering the
temperature, moisture saturation and pressure distributions in the particle. The model equations are solved numerically based on
physical properties of apple. The heat and mass transfer mechanisms in the #uidized-bed drying process are analyzed. The results
show that capillary #ow and vapor di!usion play di!erent roles in moisture transfer in the particle during di!erent drying periods.
The internal heat transfer can greatly a!ect the drying process while the e!ect of gas pressure distribution is insigni"cant. Due to the
coupled e!ects between gas and particles, the state of gas in the #uidized-bed changes substantially along the bed height and a!ects the
heat and mass transfer in the particle signi"cantly. A new parameter called bed area factor is derived and analyzed. It is important in
determining the drying e$ciency in the design and operation of #uidized-bed dryers. The e!ects of particle parameter and inlet gas
conditions on heat and mass transfer in the #uidized-bed drying process are discussed through the analyses of drying characteristics. ( 2000 Elsevier Science Ltd. All rights reserved.
Keywords: Bed area factor; Dehydration; Mathematical modeling; Porous media
1. Introduction
Due to the high heat and mass transfer coe$cients and
the large exchange area between the particles and gas,
#uidized-bed drying has a high drying rate and a short
drying time. Its use for granular materials is now well
established, and there are numerous #uidized-bed dryers
operating in the food and chemical engineering processes. In contrast with this industrial development, the
fundamental research on #uidized-bed drying has not
made parallel progress. The design of an industrial
#uidized-bed dryer is still very much an art based upon
empirical knowledge (Hovmand, 1995).
There are a signi"cant amount of works on the twophase dynamics of particles and gas as well as heat and
mass transfer between them conducted for the #uidizedbeds (Kunii & Lenvenspiel, 1991; Kwauk & Li, 1996).
Many experimental studies have been carried out on the
0009-2509/00/$ - see front matter ( 2000 Elsevier Science Ltd. All rights reserved.
PII: S 0 0 0 9 - 2 5 0 9 ( 9 9 ) 0 0 4 4 6 - 7
1858
Nomenclature
St
h
a ,a ,a
1 2 3
A
P
A
B
b ,b ,b
1 2 3
c
c ,c ,c
1 2 3
St
m
D
d
P
f
f
A
f
h
f
m
h
H
*H
IQ
m
j
j
K
D
K
r
N
Nu
P
P
!5.
P
c
Pr
q
q
r
R
g
R
v
R
P
Re
RH
S
S
#3
Sc
Sh
*
1
*
2
*
3
u
<Q
f
<
P
=
z
Greek letters
a
h
a
m
e
e
B
j
k
o
p
q
q
d
Subscripts
f
g
in
l
out
s
v
0
over bar
gas in #uidized-bed
gas in the material
inlet
liquid
outlet
solid matrix
vapor
initial
average value in #uidized-bed
1859
Gas:
L(e o )
g v "!+ ) j #IQ ,
v
m
Lq
L(e o )
g g "!+ ) j #IQ ,
g
m
Lq
Liquid:
L(e o )
l l "!+ ) j !IQ .
l
m
Lq
(7)
(8)
(9)
(10)
(11)
(12)
(13)
one1 by
2. Mathematical modeling
2.1. Heat and mass transfer in a particle
Based on the Darcy's law and Fick's law, the mass
#uxes of vapor, gas and liquid in the porous material can
be expressed as
K
j "! g o ) +P !D e ) +o ,
v
g
v g
v
k v
g
K
j "! g o ) +P !D e ) +o ,
g
g
g g
g
k g
g
K
j "! l o ) +P .
l
l
k l
l
(1)
(2)
(3)
1860
A
A
B
B
A
A
B
B
LS
L
1 L
1 L
LS
"
a r2
#
a r2
,
a
1 Lq r2 Lr 2 Lr
r2 Lr 3 Lr
(14)
L
L
LS
1 L
1 L
b
"
b r2
#
b r2
,
1 Lq
r2 Lr 2 Lr
r2 Lr 3 Lr
(15)
LP
LS
L
g "c
c
#c
.
1 Lr
2 Lr
3 Lr
(16)
(17)
(18)
L
Lr
"0,
(19)
"0.
(20)
r/0
r/0
(22)
where
<Q "uA .
f
B
"D P #( !D P ) e~fh ,
f*/
r/R
f065
r/R
o
"o D P #(o !o D P ) e~fm ,
vf065
v r/R
vf*/
v r/R
where
(24)
(25)
f "St ) f ,
(26)
h
h A
f "St ) f ,
(27)
m
m A
NA
P .
(28)
f "
A
A
B
Considering the total heat and mass balances between
the particles and gas from the inlet to outlet, the average
temperature and vapor density of gas #ow can be calculated and used as reference quantities in the present
study. Since
a A (M !D P ) N"!o c <Q ( ! ), (29)
h P f
r/R
f f f f065
f*/
a A (o D P !o6 ) N"<Q (o
!o ),
(30)
m P v r/R
vf
f vf065
vf*/
substituting Eqs. (24) and (25), respectively, into Eqs. (29)
and (30), one obtains
1!e~fh
,
(31)
f
h
1!e~fm
.
(32)
o6 "o D P #(o !o D P )
vf*/
v r/R
vf
v r/R
f
m
With and o known, the relative humidity of gas can
vf
be determined.
M "D P #( !D P )
f
r/R
f*/
r/R
(21)
(23)
Nu"2#1.8Re1@2Pr1@3,
(36)
Sh"2#1.8Re1@2Sc1@3,
(37)
1861
Table 1
Physical properties of apple
Symbol
Value
Unit
Reference
c
g
c
l
c
s
1006
4180
1810
J/(kg K)
J/(kg K)
J/(kg K)
D
*H
K
D
S
#3
e
2.56]10~5
2.44309]106
1]10~19
0.3
0.7
m2/s
J/kg
m2
*
*
j
g
j
l
j
s
k
g
k
l
0.025
0.65
0.78
1.83]10~5
0.458509!5.30474]10~3
]#2.31231]10~5]2!4.49161
]10~8]3 #3.27681]10~11]4
1.29
1000
1600
0.121978!0.0001683]
J/(s m K)
J/(s m K)
J/(s m K)
kg/(m s)
kg/(m s)
kg/m3
kg/m3
kg/m3
kg/s2
o
g
o
l
o
s
p
3. Physical properties
In the present work, the physical properties of apple,
Table 1, are used in the simulation. All the data were
obtained from credible references except K and S . The
D
#3
value of K was selected as 10~19 m2 because it is a typiD
cal value for similar fruits. S "0.3 was assumed in this
#3
calculation according to the experimental data of similar
material (Wang & Tu, 1995). The heat capacity and
thermal conductivity are obtained using the volume average method as
oc"o c eS#o c e(1!S)#o c (1!e),
(38)
l l
g g
s s
j"j eS#j e(1!S)#j (1!e).
(39)
l
g
s
On the basis of Kelvin's equation, the vapor density in
the material is
P()
o "
e~Pc @ol Rv T,
(40)
v R
v
where P() is the saturated vapor pressure function of
temperature and the capillary pressure can be written as
(Leverett, 1941)
e
P "J(S)p
.
c
(41)
K
D
The Leverett function J(S) was obtained by Perre and
Moyne (1991) as
0.020023
0.009547
J(S)"
#
!0.12S#0.4415.
S
S!1.028
(42)
K "K K ,
l
D rl
(43)
K "K K ,
g
D rg
(44)
K "
rl
S!S 3
#3 , S'S ,
#3
1!S
#3
0,
S)S .
#3
(45)
(46)
4. Numerical results
4.1. Heat and mass transfer for a typical operation
4.1.1. Heat and mass transfer in a particle
Eqs. (14)}(20) and (31)}(35) were solved numerically
with the "nite di!erence method. The typical operating
conditions are listed in Table 2. The numerical error was
tested with various grids. The grids of 200 were selected
because only less than 0.1% di!erence was found between the results obtained with the grids of 200 and 400
for the typical operating conditions.
1862
Table 2
Typical operating conditions
Symbol
Value
f*/
RH
*/
d
P
f
A
u
P
!5.
0
S
0
803C
10%
2 mm
10
2 m/s
1.01325]105 Pa
203C
1
Fig. 3. Pressure pro"les in the particle during drying. q(s): 1}0; 2}5;
3}30; 4}60; 5}90; 6}120; 7}150; 8}180.
Fig. 2. Saturation pro"les in the particle during drying. q(s): 1}0; 2}5;
3}30; 4}60; 5}90; 6}120; 7}150; 8}180.
1863
1864
Apparently, larger temperature di!erence in the particle will cause greater deviation of the lumped temperature model from the distributed parameter model. Such
a large temperature di!erence can be created either by
a small thermal conductivity of the solid particle, or
a large particle diameter. For a material with thermal
conductivity of 0.078 W/(m K), it takes much longer time
than for apple as indicated by curves 1 and 2 in Fig. 5.
The calculation results in the following part of this work
show that it will take more than 3.5 times long time to
dry the same weight of wet particles at diameter of
5 instead of 2 mm.
It is interesting to see that the distribution of gas
pressure in the thermally less conductive particle, Fig. 6,
is very much di!erent from that seen in Fig. 3. During the
initial period, the pressure at the particle center is slightly
higher than that at the surface. Thus, the gas in the
capillary region #ows from the material to the surrounding. Then the inside pressure close to the surface becomes
negative and a minimum pressure was predicted which
means that the gas #ow is in the direction of moisture
#ow near the particle center while opposite to this direction near the surface. With the gas #owing from the
surface to center at the end of drying, the pressure distribution approaches uniformly.
of heat transfer in the #uidized-bed dryer and the capacity of gas to supply heat in the #uidized-bed. As for
moisture transport in the #uidized-bed dryer, the average
and outlet relative humidities of gas are used in the
following analyses.
Fig. 4 also shows temperature variations of the gas
during drying. The gas temperature drops from 803C at
inlet to about 503C at outlet in the "rst falling rate period
and the di!erence * is more than 303C. It indicates
3
that the heat transfer intensity is very high accompanied
by a high drying rate. In the second falling rate period,
* keeps decreasing which suggests that the heat ex3
change intensity becomes weaker although the capacity
of the gas to supply heat gets larger.
During the drying process, heat transfer resistances in
the bed include the coupled internal heat transfer resistance in the particle and external heat transfer resistance
between the particle and gas. In Fig. 4, it is seen that
during the "rst falling rate period, * is almost zero
1
while * is more than 153C. Obviously, the heat trans2
fer is externally controlled in this period. When the drying is in the second falling rate period, * increases
1
until shortly before the end of drying while * de2
creases all the time until it reaches zero. At about 128 s,
both * and * have the same value. Thus, it can be
1
2
concluded that both the internal and external heat transfer resistances control the drying process in the second
falling rate period. This is in accordance with the e!ect of
temperature distribution analyzed previously.
The predicted mass transfer behavior is consistent with
that of heat transfer. Fig. 7 shows the variation of gasrelative humidity during drying. It is impressive to note
that the outlet-relative humidity is more than 40% during the "rst falling rate period. During the second falling
rate period, the outlet-relative humidity keeps decreasing
according to the temperature variation. The "gure also
1865
(47)
Table 3
Drying times at di!erent f
A
f
A
q,s
d
q /f , s
d A
0.1
1
10
100
1000
109
113
163
940
9020
1090
113
16.3
9.4
9.02
1866
Table 4
Drying times at di!erent d
P
d , mm
P
5
2
1
0.5
0.2
0.1
f "10
A
="3.93 kg/A
B
=, kg/A
B
q,s
d
f
A
q,s
d
total q , s
d
9.83
3.93
1.97
0.983
0.386
0.197
688
163
62
26
9.4
4.6
4
10
20
40
100
200
609
163
101
92
90
90
275
163
124
104
94
92
1867
ing into the #uid bed dryer. Fig. 11 shows that the drying
rate increases greatly with the inlet-relative humidity
decreasing. Therefore, comprehensive optimization
should be carried out between reducing drying time by
decreasing the air humidity and conserving energy by
reusing the outlet hot air.
Considering the product quality, the maximum tolerable temperature by the material is usually employed as
the inlet gas temperature in practice. Here, an absolute
humidity value of 0.02 (kg water/kg dry air) is used in
order that the drying is available under the conditions in
the range of 40}1003C for this simulation. The calculation shows that although the particle surface temperature rises quickly during the second falling rate period
and the material may be damaged by overheating
for higher inlet air temperature operations, the particle
1868
surface temperature remains small for a rather long period. Therefore the inlet gas temperature can be of a high
value initially and changed to the maximum tolerable
temperature afterwards. In this study, 603C is considered
as the safe temperature for apple. At "1003C, the
f*/
particle surface temperature is not more than 603C until
q"47 s when 60% of the total moisture in the particle
has been removed. While for "803C, hot air can be
f*/
used for 92 s and 77% of the moisture is removed during
this time. If the maximum tolerable temperature 603C is
used as the inlet gas temperature, the time to remove 60
and 77% moisture is, respectively, 112 and 160 s. Thus it
establishes that biomaterials can be dried faster and
retain good quality using high drying temperature, provided that the hot gas is used for the right amount of
time. The present model provides a useful tool for the
determination of this time value.
5. Conclusions
Di!erent moisture transport mechanisms in the material play di!erent roles in di!erent drying periods of
#uidized-bed drying of moist porous particles. The lumped temperature model is not valid in #uidized-bed drying of moist porous particles because of the signi"cant
internal heat transfer resistance, especially for low thermal conductivity materials. However, the pressure distribution e!ect on heat and mass transfer in drying is
insigni"cant. The transport processes in the particle are
signi"cantly a!ected by the coupled heat and mass transfer between the particles and gas in the #uidized-bed.
A new variable called bed area factor is derived from the
di!erential equations and its potential in the design and
operation of #uidized-bed drying is demonstrated. With
the increase of the value of this bed area factor, the e!ect
of "niteness of gas becomes signi"cant. However, the load
of materials should be increased to raise the drying e$ciency when the bed area factor is small. For a given load
of particles, the drying time reduces with particle diameter
decreasing until a critical value is reached. Temperature
programming can signi"cantly shorten the drying time of
biomaterials while retaining the product quality.
Acknowledgements
The authors are grateful for the "nancial support from
BRI of HKUST and ISF Fund of H.K.S.A.R. Government
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1869
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