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NYO-1576(DEL.)
P r e s e n t e d by
The S t a f f , Health and Safety D i v i s i o n
M e r r i l Eisenbud, D i r e c t o r
J a n u a r y 2 8 , 1952
LEGAL NOTICE
This report was prepared as an account of Government sponsored work. Neither the United
States, nor the Commission, nor any person acting on behalf of the Commission.
A. Makes any warranty or representation, expressed or implied, with respect to the accu-
racy, completeness, or usefulness of the information contained in this report, or that the use
of any Information, apparatus, method, or process disclosed In this report may not infringe
privately owned rights; or
B. Assumes any liabilities with respect to the use of, or for damages resulting from the
use of any information, apparatus, method, or process disclosed in this report.
As used in the above, "person acting on behalf of the Commission" Includes any em-
ployee or contractor of the Commission, or employee of such contractor, to the extent that
such employee or contractor of the Commission, or employee of such contractor prepares,
disseminates, or provides access to, any Information pursuant to his employment or contract
with the Commission, or his employment with such contractor.
M
DISCLAIMER
HY0-IS7C
SUMMARY 6
INTRODUCTION 7
GENERAL DESIGN OF THE MONITORING PROGRAM 8
ORGANIZATION 10
METHODS OF FIELD OPERATION 12
Phase A - The Weather Bureau Network 12
Aenal Observations Along the 85th Meridian 16
Phase B - Mobile Monitoring 19
Operations on the 9^th Meridian 19
Aerial Observations on the 95th Meridian 20
Mobile h o rtonng for Operation JANGLE 20
METHODS OF LABORATORY STUDY 24
Sample Processing S>4
Counting Procedures 24
Calculations and Reports 2%
Extrapolating 2S
FINDINGS 31
Natural Radioactive Background «?'
Fallout During the Pre-test Period 31
Observations from the Weather Bureau Network During Operations BUSTER and JANGLE 33
Mobile Monitoring for Operation BUSTER 4o
Aerial Observation* Along the 95th Meridian (low level) 40
Aerial Observations Along the 85th Meridial (nigh level) 40
Mobile Monitoring During Operation JANGLE 4?
-vtial JANGLE Det mation 4J
Second JANGLF Detonation 47
Relationship of Findings to Criteria of Jangle Feasibility Committee 47
THE PROPERTIES OF FALLOUT SAMPLES h4
Particle Size 54
Radioactive Decay '4
Absorption Measurements 84
Radioautographs of Settled Dust %6
NOTES ON FIELD TECHNIQUES 89
Comparison of Tray and Gummed Paper Techniques 69
Variation between Duplicate Trays 69
Comparison of High Altitude Measurements /?
Appendices
A.* Daily maps giving data from the Weather Bureau network for the period October 7 through December IS, 1951
(Bound Separately)
B„* Daily maps summarizing data obtained during high and low level aerial reconnaissance, and during mobile
monitoring of Operation BUSTER (Bound Separately)
C„ Equipment Provided for Weather Bureau Network (Phase A) 85
D„ Equipment Provided for Mobile Monitoring Teams (Phase B) 86
E„ Procedure for Collection of Precipitation and Dust Samples for Radioactive Fallout Studies 89
F„ Data and Summary Sheets used by Sampling Stations and Counting Laboratories 92
G. Air Samples from 95th Meridian Mobile Monitoring 94
H. Duplicate Tray Data 113
* Appendices A and B were given a limited distribution by the New York Operations Office, and is not included at
this copy of NYO-1576 ^ A C * 5 ? ^ <* »•*j?/jf-»"3^fe^
if
S
SUMMARY
The program went into operation during the f i r s t week in October in order
to permit the collection of background data for some weeks p r i o r to the i n i t i a l
t e s t of the BUSTER s e r i e s . However<> two atomic explosions in a foreign country
had occurred j u s t \ n o r to the s t a r t of t h i s program and background informs-
t i o n was thus not obtained.
During Operation JANGLE, the mobile monitoring teams were deployed at approxi-
mately 0 = 16° in the annulus of 200-500 miles from the Test Site,, For both
JANGLE detonationsj, t h e highest radioactive dust concentrations were reported
from Elko, Nevada, The 2U hour average concentration a t Elko was 1A1*,G0Q d/m/d^
following the i n i t i a l detonation and 38,000 d/m/M-3following the second detona-
tion,, The maximum values were 360,000 d/m/M^ and 180,000 d/m/hP0 The external
radiation l e v e l s associated with the passage of the debris over Elko did not
exceed 2 mr/hour„ Although these values are r e l a t i v e l y high in companion
with other data from these and previous t e s t s , the average concentrations are
very much lower than the permissible exposures established by the JANGLE
F e a s i b i l i t y Committee,,
The New York Operations Office was requested' 'by the Division of
Biology and Medicine* U,S„ Atomic Energy Commission, lftashingtonsD„C„
to coordinate a program of monitoring for radioactive fallout over
the entire United States beyond 200 miles from the test site,,
(1)
Memorandum October 8, 195l s J . C. Bugher to W. E, Kelley
04
GENERAL DESIGN OF THE MONITORING PROGRAM
(2)
v
'"Survey of Fallout of Radioactive iwrterial Following The Las Vegas,
Nevada Test Explosions" issued by the Hetlth & Safety Division,
NYOO, AEC, February ??, 1951.
(3)
' " D u s t and P r e c i p i t a t i o n Saiaj l i n g Piogram, A p r i l t h r u June 1>51"
Issued by Health & Safety D i v i s i o n , NYOO, AEC, u n d a t e d .
but only during Operation BUSTERS AT-U7 which had been made
available by the Air Materiel Command primarily for the purpose
of transporting the mobile ground observers to various s t a t i o n s
along the 95th meridian, was u t i l i z e d for observations a l o f t . In
" t h i s portion of the study, the t r a v e r s e s were made at r e l a t i v e l y
low a l t i t u d e s (2000-5000 f t . ) over the portion of the 95th meridian
straddled by the ground observers.
- 9 -
ORGANIZATION OF THE MONITORING PROGRAM
Needless to say, a study of this magnitude could not have been ac=
complished without the close cooperation of several governmental
agencies and AEC Laboratories which undertook responsibilities as
follows s
Uo S. Weather Bureau
Hanford Works
Argonne National Laboratory
Brookhaven National Laboratory
Oak Ridge National Laboratory
University of Rochester, AEC Project
University of California, AEC Project
11
METHODS OF FIELD OPERATION
Trays were exposed for 2k hour periods. The water layer was
then collected in a jar, the surface of the tray cleaned with
additional water and the combined liquids filtered through a
3 W #1*0 Whatman disc. Where precipitation occurred, the col-
lected water was processed in a similar manner.
1 Seattle, Wash. A HW
2 Medford, Oregon C HW
3 Sacramento, Cal. B UCLA
C it n
k Santa Maria, Cal.
ti ii
5 San Diego, Cal. A
6 Pendleton, Ore. B HW
7 Great Falls, Mont. C HW
8 Po catello, Idaho A HW
9 Salt Lake City, Utah C HW
10 Emery Park,(Tucson) B UCLA
Arizona
11 Bismarck, N. Dak. C HW
12 Rapid City, S„ Dak. B HW
13 Colorado Springs,Colo. C UCLA
lit Norfolk, Neb. C HW
15 Topeka, Kans. c HW
16 Oklahoma City, Okla. c ORNL
17 Abilene, Texas A UCLA
18 Corpus Christi c UCLA
19 International Falls, c ANL
Minn.
20 St, Cloud, Minn. A ANL
21 La Crosse, Wise. B ANL
22 Peoria, 111. A ANL
23 Memphis, Tenn. C ORNL
2k Texarkana, Ark. C ORNL
25 Del Rio, Tex. A UCLA
26 Sault Ste, Marie,Mich, D ANL
27 Grand Rapids, Mich, D ANL
28 Fort Wayne, Ind. D UR
29 Cincinnati, Ohio D UR
30 Lexington, Ky. D UR
31 Nashville, Tenn. D ORNL
32 Chattanooga, Tenn. D ORNL
33 Atlanta, Ga. D ORNL
3k Montgomery, Ala. D ORNL
35 New Orleans, La. C ORNL
Code
A - 1 Tray
B - 2 Trays
C - 1 Tray and Gummed Paper
D - 1 Tray & Hi-Volume Sampler
13
•:0
(Table 1 - c o n t ' d )
36 Cleveland, Ohio A UR
37 R o c h e s t e r , N.Y. B UR
38 E l k i n s , W. Va, C BNL
39 Columbia, S„ Car. c BNL
Uo Tallahassee, Fla. D ORNL
1*1 Tampa, F l a . B ORNL
k2 Caribou s Me, B UR
k3 B u r l i n g t o n , Vt. C UR
kk Binghamton, N„Y. C UR
1*5 Hartford <, Conn. c BNL
k6 New Cumberland,Pa. B BNL
1*7 Atlantic City, N.J. A BNL
1*8 A n a c o s t i a , D.C. C BNL
1*9 Norfolk, Va. A BNL
50 R a l e i g h , N. Car. B BNL
51 New York. N.Y.(NYU,AEC) C NYOO
52** B o i s e , Idaho A NYOO
53** Winneiroicca, Nev. A NYOO
51*** Reno„ Nev. A NYOO
55** Milford, Utah A NYOO
56** Grand J u n c t i o n , Colo. A NYOO
57** Alamos a, Co l o 0 A NYOO
58** Wmslow, £ri'z. A NYOO
59** Albejuerque, N.iAex. A NYOO
60** IhoenLit, A r i c . A NYOO
61** Yuma j A r i ' . , A NYOO
A -* 1 Tra>
B - 'c Trays
C - 1 Tra> ? n i Guirjnud Paper
D - 1 Tray and hi-Volume Sampler
- 11* -
'1
AEROTEC SAMPLER
& HIGH VOLUME SAMPLER
FALL-OUT TRAY
"^'^r^::^-51^^
•4 • ' " ' * '
tZ>
i'
. pant,
\
, ^ _ ^ ^ S f ^ FALL-OUT COLLECTION EQUIPMENT USED •
«S3.
IN GROUND SAMPLING OPERATIONS. »v«i^*4fc.>- s.1 \
The equipment was located at positions convenient to the Weather
stations. Trays were placed on the ground outside the buildings
or on flat roofs. Hi-Volume samplers were placed on pedestals on
the ground with protective enclosures around them or in open windows
in balloon sheds or otherwise infrequently used buildings.
In most cases, samples were changed just after midnight when the
duties of the man on this shift were fairly light. At this time,
Hi-Volume filters were changed and the tray samples were collected
and filtered. The entire operation could be completed in from ten
minutes to a half hour, depending on the types of equipment at hand.
The B-2?s were provided by the Air Weather Service and were of a mod-
ified type, equipped with radioactive monitoring equipment. Thess
are normally in continual use by the Air Weather Service. The equip-
ment consisted ofs
- 17 -
4
,-*\
«Hft?fc*t ^ ^ift^W.^
f * u * •*'«>f-f*'«ptM<r»)^t^w^g
FIG. 2
m^ihitilliltewir''if-rt-MfV^*^^-^a>... ,,
RCL GM TUBE FiTtEO WITH SPECIALLY MODI-
FIED BATTERY OPERATED RATE METER.
The two Health and Safety members supervised the setting up of ground
stations operated by the airmen, set up and operated their own stations,
and operated sampling equipment in the C-l*7 during survey flights. The
- 19 -
«;
equipment was similar to thst provided the Weather Bureau stations,
A ^B but in addition, instruments for particle size differentiation were
made available. A course separation of airborne particulates into
two fractions above and below approximately 5 microns.in diameter-
was achieved by mounting an Aerotec in front of the Hi~Volume sampler.
This unit is essentially a small Cyclone dust collector which at its
rate of capacity of 1*5 c.f.m. is efficient in collecting of particles
larger than approximately 5 microns. The large diameter fraction
separated by the Aerotec was analyzed separately from the small
diameter fraction which was collected on the filter paper of the Hi-
Volume air sampler.
When time permitted, the C-li7 was utilized for the collection
of radioactive dust at altitudes of 2000-5000 feet. Hi-Volume air
samplers were mounted in the cabin of the C—1*7 in such a manner as to
sample the heating air emitted at the air duct vents. This air is
drawn into the system through scoops mounted on the wings. Cascade
Impactors and a Halross Scintillometer were also available.
In general, the plane would traverse the 95th meridian between air-
fields at which the mobile ground observers were based.
Seven members of the Health and Safety Division and five airman, opera-
ting in teams of two, set up six ground stations for the first test.
For several days prior to the test, this group was based at Indian
Springs Air Force Base, Nevada, awaiting orders to sampling locations.
Immediately after the detonation, wind data were evaluated and sampling
locations were selected by an Air Force meteorologist and a Health and
Safety representative at the test site. Within an hour, the teams were
airborne, with instructions to establish stations at Delta, Salt Lake
City and Wendover, Utah, Elko, Nevada and Burley and Idaho Falls, Idaho.
Equipment was set up and sampling started at each site iranediately upon
arrival. Sampling continued for about 2l* hours.
For the second JANGLE test, stations were each manned by one Health
and Safety Division member. Since it was expected that south to
southwest winds would prevail, perspnnel.were based at Ogden Air Force
Base, Utah, prior to the test. A H&S representative at the Test Site
telephoned instructions to the team at Ogden when the estimated traject-
ory' became available shortly after the detonation. The C~i*7 was
- 20 -
.. 4
dispatched, leaving teams j»t Ogden, Prove (Utah), Delta, Rock Springs
(Wyoming), Wendover (Utah) and Elko (Nevada). The locations of
sampling stations are given in Figure 3. Sampling for the second
JANGLE test continued for approximately 36 hours.
Each ground observation station was equipped with the following ap-
paratus?
The 2610A and Zeuto were used for the direct measurement of ground
activity. The two instruments provided a wide range of sensitivity.
The areas -iround the stations were scanned at frequent intervals with
the meters held about 3" above the ground. Spots of high activity
were measured by the less sensitive Zeuto.
A special probe (Figure 1*) was developed for the 2610A to measure
activity on filter papers. This device enabled the use of a method
of sampling which reduced the total number of Hi-Volume samples collected
by cutting down the frequency of collection during periods of low
activity. This eased the task of the team membersyand more important
saved laboratory time later on. Repeated readings were made of the
sample on a single Hi-Volume filter paper collected over several hours
until an increase in airborne activity was detected. At that time,
a 20 minute sampling period would be established. Measurements were
then made each 20 minutes as the samples were changed until the activ-
ity decreased to its original value. Continuous sampling on one
filter was than resumed.
When activity on filters exceeded the high range on the 261OA^, the
Zeuto was used. An extrapolation determined in the field permitted
reliable transition from one instrument to the other.
- 21 -
/ S
Z*? %*•'
*\ _' 0
0- u I
v
- ^ J' £ *» »£ " \- s ' Jr Jag? •- > »»&
:
A * * t S ^ > ' ( ^ \ i * \f**& SYMBOL TEST DATE ,
FIG. 3
DISTRIBUTION OF MOBILE GROUMO STATIONS
FOR JANGLE SERIES OF TESTS
22 -
019
-
WS
FIG. *
Sample Processing
All samples were ashed before counting. Whatman filter paper samples
were ashed with the cellophane bag, while the gummed paper and air-dust
filtir samples were ashed without the bag. The Whatman and air-dust
filters were used as received. The gummed papers were sampled by
cutting out l/U square foot from the center of the paper.
Counting Procedures
2U
,?j
E. Standardizations The efficiency factor for converting
net counts per minute into d/m was obtained by meas-
uring the counting rate of an NBS standard of RaD
and RaE plated on a palladium coated silver disc. The
disc diameter is 308 cm and the active area has a dia-
meter of 2 si; cm. A standard having a disintegration
rate of 5000 to 50,000 was supplied to each laboratory.
The factor of c/d was obtained by running the standard
for 6it,000 total counts. The usual factor was about
0.08 c/d.
v
5«
the fallout from other tests effectively nullified this
system, and arbitrary levels had to be taken to judge
significance.
Summary sheets were provided for tabulating the data from each site.
One sheet was used for each type of sample at a single site counted
during a week.
Samples of the data sheets and summary sheets used are included ss
Appendix F.
Extrapolating
26 -
• I
EXTRAPOLATION FACTOR
FROM COUNTING DATG TO SAMPLING DATE
Days-Bus t Days - Burst to Sampling
to Count
The burst date corresponding to fallout at a given sampling station
on a given day was selected by consideration of the unextrapolated
results for the tray samples collected at each station. These results
were tabulated by day and by station on daily maps. Significant in-
creases in activity were marked on the map, and by consideration of
results in different areas, the course of the fallout for a given
burst was charted. Gummed paper and air-dust samples were used only
for confirmation.
The extrapolated values were recorded on daily maps and the assumed
burst noted for each sample.
- 28
',ri
TABLE 3
FACTORS FOR EXTRAPOLATION FROBII SAMPLING DATE TO FEBRUARY Z ~ l t
D a y s -Burst
Burst 10/88 B u r s t li3/%!8 B u r s t 10/30 B u r s t 11/1 Burst 1#9 B u r s t 11/29
0004
o 008
,004
0010
oooh
.010
0
0
004
010
Q006
00x3
..016
007
003.4 .oa6 ,016 om6 0 021 * 026
s 026 0022 0022 .023 0 050 0%
o,
0 026 0 029 .O30 .o3a oohro 048
0032 00% o 036 e 038 0049 .058
n 038 0043 ,044 0 045 0 059 0070
9045 .o50 0852 0 05.3 0 070 ,085
0052
e858
0
.a
0% 0
eo66
059 006% e080
089 .
0095
nop
.
Q
o
0
132
15%
m
0135
.a5
0
0.40
150
.16o
e 182
* 195
a208
e23.7
0233
-248
enWc ,$62 .165 e 171 *222 P265
03.55 0 170 0 g73 -el79 8233 ,278
0 159 e 178 e 182 o 188 6245 0292
,165 e 185 0199 f* 0254 03sbc
0175 e a* e200 0208 0269 ,520
e 185 0208 0212 SZO 02134 Q340
Table U
30 -
FINDINGS
Daily observations obtained from the Weather Bureau network are given
in Appendix A. As noted earlier, it was to have been a period during
which background measurements would be recorded, but the occurrence
of atomic explosions in a foreign country conspired to vitiate this
portion of the study. Positive indications of activity were reported
from the very first of our collections. Beginning on October 7 and
continuing until October 21 we find positive but low level indica-
tions of radioactivity. The values are low in comparison with the
data to be reported when Operations BUSTER and JANGLE were in progress.
31
Table 5
Cleveland., Ohio 28
Rochester, N.Y. (U.of Rochester) 22
Rochester, N.Y. (Eastman) 89
Boston^ Mass. 29
Upton, N.Y. 15
32
»(»
One sample of dust collected from the high volume sampler at Fort
Wayne, Indiana, on October 11-12 was studied for decay characteris-
tics. If the decay is assumed to be the usual fission product form,
with a slope of -1.2, then the estimated date of the burst from which
this sample originated would be September 2l+.
The occurrence of radioactive debris from other than the Nevada Test
site served to confuse our monitoring program from the start. It
proved to be an additional complication in a study which from the
outset was beset by innumerable difficulties.
The daily maps giving all data reported from the Phase A Weather
Bureau network are given in Appendix A. In coordinating the
collection and counting of samples and in putting the data into
useful form, the purpose for which this survey was undertaken has
been largely served. There remains a requirement for extensive
meteorological analysis of the information. It is to be hoped that
when this is accomplished cooperatively by the U. S. Weather Bureau
and the U. S„ Air Force, there will accrue a better understanding of
the fundamental phenomena involved in fallout.
E>« ,
ZOO
90\
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no &20
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e -~jf
^2° [Tool 920
//OO
/-eo
\29$ So
«o
'Jfl »j?/r
eo
\27
o
JH t
j/'fad'
,ESc
1/70 \ ©/•*
340' 580
JO 380. L7 « o
AW
3&*
'50 oao
/3® 730
fso Jo \S90\
Z9C
0 \
ft 32$ 39°
I O/fi 4901
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| ZGO\s -»20 \eeo
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>o<2>\zZd\\
'7o.
o40
# lS»
yfi
lHH]
Fig. 6
/SO/ 170
CUMULATIVE FALL-OUT FROM ALL
BUSTER AND JANGLE TESTS EX-
TRAPOLATED TO FEBRUARY I , 1952.
d/m/ftz/<£uj TRAY
FALL-OUT M M I TOD I He
0 GUMMED PAPER
HEALTH ANO SAFETY DIVISION
NED YORK OPERATIONS OFFICE at/m/meter3 * AIR FILTER
U . S . ATOMIC ENERGY COMMISSION
85°
/os°\ J 95"
will have a half life of "approximately three months. The
community which is next highest is Norfolk, Virginia with
2200 d/m/ft2$ about one-fifth of the Rochester value. A
large number of communities along the east coast report
cumulative values of 1000 d/m/ft2.
2. The total activities, both from the Nevada test and from
fallout of foreign origin, are given in Figure 7» In the
area of maximum deposition, the eastern half of the United
States, the foreign contribution is only slightly signifi-
cant, but it will be observed that in northwestern U. S.
the foreign contribution to the total is more prominent.
*.N
Fig. 7
TOTAL FALL-OUT
Oct. 7 TO Dec. 15, 1951
EXTRAPOLATED TO Feb. I , 1952
dlmlft'ld^ TRAY
0 GUMMED PAPER
FALL-OUT MMITMIM 3
HEALTH AHD SAFETY D I V I S I O N at/m/meter # AIR FILTER
DE» YOIK OPERATIONS OFFICE
U . S. ATOMIC ENEROY COMMISSI OK
10s
Fl gure 9
10"
I0J
10'
10
39
jr.
Mobile Monitoring for Operation BUSTER
Table 6 gives the data collected aloft by the C-i+7 traversing the
95th meridian between coraiaunities at which mobile stations were
located. As in the case of the ground level samples, the values
are surprisingly low considering that these traverses were presum-
ably made beneath the main cloud body. On the other hand, as noted
elsewhere in this report, the data are suspect because of difficulties
in obtaining representative air samples on the C—1+7 flights.
- UO -
TABLE 6
The area west of Elko should have been included in the survey,as
shown by the sharp increase in activity between Wendover and Elko.
Our data do not define the most western extent of fallout zone. The
best available estimate of the trajectory indicated that in the posi-
tions shown our teams would be astride the fallout zone on the line
from Salt Lake City to Elko. That this was not the case is clear
from the data.
The maximum dust concentration had probably passed by the time Elko
collections were started. The first sample collected for 20 Jiinut.es
beginning at 1630 M3T was the highest value reported, j60,000 d/ra/M^.
Thereafter, the airborne activity rapidly declined to well under 100 d/m/M^
at 0200 the following morning. For the 2l+ hour period the average
concentration was 1+1+,000 d/uiin/M?taking the means of all samples wimh
the result of each sample extrapolated to the midpoint of its indivi-
dual time of collection. The mean age of this dust may be taken as
approximately 10 hours.
As will be noted from Table 7> the bulk of the activity was contained
in particles less than 5 microns in diameter. The one exception was
the Aerotec sample at Burley where the bulk of the activity was included
in particles larger than 5 microns in diameter. This is in 'contrast,
not only to the data from other stations, but to the results of
Cascade Impactor samples of Burley air collected at the same time as
the Aerotec sample.
- 1*2 -
TABLE 7
Ave. Type
Place Monitoring Period Highest Sample Cone** Collector Total Fallout
Time Cone* Cascade Aerotec
(d/m/M3) (d/m/M3) Impactor d/m/ft.'
Elko, 19 Nov. 1630 - 20 Nov. 1100 19 Nov. 380,000 kk,000 90 82 Tray 110,000
Nev. 16U0 Gummed Paper 59*000
to 1700
1 Wendover, 1 9 Nov. 1630 - 20 Nov.1100 19-20 Nov. 3,000 1,000 Tray 220,000
,-*=: Utah 2000 Gummed Paper 105,000
eo
to 0600
1
Idaho
Falls, 19 Nov. 20U5 - 20 Nov.0800 20 Nov. 3,000 koo Tray k,100
Idaho 0000 Gummed Paper 120,00
to 0100
:
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The tray activities are lower than would be expected, considering the
high concentrations of airborne dust. During Operation JANGLE, as
during BUSTER, the relationship between air-borne and settled dust
was not as would be expected„
The highest external radiation level observed by the mobile teams was
2 mr/hour at Elko. This level had been reached when the mobile team
arrived at 135>0 on 19 November.
kl =
TABLE 8
Elko, 29 Nov, 1720 - JO Nov. 2230 30 Nov. 190,000 38.000 >95 Tray Lost
Nev. 0600 Gummed P a p e r 210,000
Ogden, 29 Nov, 1900 - 30 Nov. 1900 30 Nov. 710 205 81+ Tray 1,300
Utah 0100 Gummed Paper 9.700
Wend over, 29 Nov, 161+0 - 1 Dec, 001+5 1 Dec. 1+.300 2,200 77 65 Tray 60,000
Utah 00l+5 Gummed P a p e r 7,000
' Delta, 29 Nov, 1100 - 30 Nov, 1110 29 Nov, 550 185 92 Tray 81+0
£ Utah 1100 Gummed P a p e r 30,000
1
Rock Springs
Wyoming 29 Nov, 121+5 - 30 Nov, 2250 30 Nov, 2,800 85 9U Tray 1,300
1U50 Gummed Paper 50,000
Provo, 29 Nov, 1915 - 30 Nov. 2020 30 Nov. 5,1+00 190 83 Tray 1,000
Utah Ql+20 Gummed Paper 11,000
* E x t r a p o l a t e d t o time of c o l l e c t i o n
** Ave. of i n d i v i d u a l samples e x t r a p o l a t e d t o time of collection
= ; RADIDACTiyE DUST FRpM T E I T 0 N ?9 NOVEMfifeft
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(HOURS - M S T )
29 NOVEMBER 3 0 NOVEMBER
- 53 -
40
THE PROPERTIES OF FALLOUT SAMPLES
Particle Size
Radioactive Decay
A
2 = AX ( ^ )
where A£ and A-j_ are the activities at times t2 and t]_ after fission.
-ft _
-I
FIG. 18
Explosion Key
5
\ November 29, 1951
4
_ 95
_ 90
75 E
50
— 25 S
_ 10
I
nr I 0.5 0.1
PARTICLE DIAMETER (MICRONS)
- 55
M I1
• i ,<
I 0.5
56
Hunter and Bailout)have calculated the individual and total beta
activities produced in a U235 atomic explosion. In the time range
of 1 to 100 days, the Way and ilifigner expression is shown to be valid
as far as decay rate is concerned.
Figure 20 shows how a decay following the -1.2 exponent would behave
if the burst were misjudged by two days in either direction. If
the burst was assumed to be two days earlier than the true time., a
straight line through the later points would have a slope of XL„37s>
while the opposite error would give a slope of -1.06.
If the sample is counted within three or four days after the burst
and the decay follows the -1.2 exponent, it should be a simple
process to place the burst time to the nearest day. However;, it is
apparent from Table 9 that the decay rates vary widely. The general
use of decay rate for selection of burst date is subject to great
error, particularly if the normal counting error is taken into
consideration.
Some of the samples whose decay rates were measured had been subjected
to particle size separation with a Cascade Impactor or Aerotec unit.
The results on these samples are tabulated in Table 11„
All indications from these scattered results are that the larger
particles decay at a greater rate than the smaller particles. This
factor may be slightly complicated by the presence of induced activi-
ties, but this effect should not be large after a few days, unless
the fraction of induced activity in the sample is very large.
= 57 _
TatiTeT"
-58
Table 9 (Cont'd.)
$9 -
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Table 9 (Cont'd.)
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- 62 -
Table 11
Burst Decay
Location Date of Sample Bate Slope
-63 -
Absorption Measurements
The results on the decay rates of the components are given in Table 12,
Absorption data on other samples were obtained but decays were not
run. All showed similar components.
6k -
^J
Table 12
65 -
Radioautographs of Settled Dust
Duplicate gummed papers were exposed on the roof of NYO during the
swvey period. One of these samples was processed and counted,
while the other was radioautographed to determine the distribution
of radioactive particles.
- 66 -
67
'4 /
Table 15
5 640 4.0
6 2500 4.0
7 3000 6.0
S 540 3.0
9 6900 6.0
10 2200 5.0
11 520 2.8
12 470 2.9
13 570 2.0
14 2000 4.0
lw 870 2.7
16 660 3.5
68
NOTES ON FIELD TECHNIQUES
A similar comparison was made of data for days when more than
a trace of rain was reported. Figure 23 is the logarithmic plot.
In this case, also, the gummed paper collected the more activity
and the regression coefficient was highly significant. The re-
lationship between tray and gummed paper data is essentially the
same in rain and fair weather. That is5 the differences between
corresponding coefficients in the equations are not significant
statistically.
The precisions of the two methods have not been compared. Such
a comparison would entail replication of both at the same loca-
tions. Both methods may be subject to inaccuracies which the
data cannot reveal. It appears possible, for instance, that the
gmnmed paper may overestimate the fallout by collecting dust
blown from nearby surfaces. This source of inaccuracy might be
investigated by comparing gummed papers located at different
heights.
- 69 -
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- 70 -
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l t Q
71 -
Comparison of High Altitude Measurements
Dust filtered out of air at high altitudes was tested with an ItCL
GM tube as described previously. These measurements were made on
the plane but after its return to the base the activity of filter
paper was determined with a laboratory beta counter,) The results
by the two methods are plotted on logarithmic Scales in Figures 2k
and 25o The points of Figure 2k $ representing activities below
1000 counts per minute, give the impression of random scatter rather
than correlation. Above 1000 counts per minute the results of the
two measurement methods are clearly correlated,, These data and
the regression line are plotted in Figure 2f>. (The regression
coefficient is highly significant.)
The relation between the filter paper activity and the readings
of a scintillometer and a conductivity meter was investigated.
An inspection of the time graphs (Figures 26 - 33) indicates that
there is a rough correlation among the three sets of data. There
are peaks in the curves which appear to correspond, but they do
not coincide in time. Rather, there are irregular lags which
prevent the pairing of the data and make the use of statistical
methods of comparison difficult. Some of the peaks in the instru-
ment readings are accompanied, usually with a time differencesby
rises in filter paper activity, but there are other conductivity
and scintillometer peaks with no corresponding change in the filter
paper.
- 72 -
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APPENDIX A*
(Bound Separately)
83
APPENDIX B*
(Bound Separately)
-8k
APPENDIX C
1 Tray
1 Squeegee
1 Kit of equipment for filter samples
70 Data Sheets
1 Set of Instructions
70 Addressed franked envelopes
(addressed to the local analytical lab)
70 Plastic sample envelopes
2 Trays
1 Squeegee
2 Kits
140 Data Sheets
1 Set of Instructions
70 Addressed franked envelopes
140 Plastic sample envelopes
1 Tray
1 Squeegee
1 Kit
140 Data Sheets
1 Set of Instructions
70 Addressed franked envelopes
140 Plastie sample envelopes
1 Frame for gunmed papers
70 Sheets of gummed paper
1 Tray
1 Sqtteegee
1 Kit
140 Data Sheets
1 Set of Instructions
70 Addressed franked envelopes
140 Plastic sample envelopes
1 Hi Volume Sampler
70 4 W diameter dust filters
70 Addressed envelopes (addressed to NYOO)
- 85-
APPENDIX D
Noo of Items
per Team
86
P4i
APPENDIX D (Con't)
E - Hi Voluire Sampling K i t
1 Carrying Case
1 E x t e n s i o n Cord 50"
1 Cube Tap
2 Boxes hn Whatman #L|1 F i l t e r Paper
2 Boxes Comfo A l l Dust F i l t e r s (100)
300 Cellophane Sample Envelopes
1 P a i r Forceps
1 Glass Marking P e n c i l
300 Data Sheets
25 L a r g e , Addressed, Franked Manila Envelopes
2 Hi Volume Samplers
k Hi Volume Sampler Heads
h 3-Wire F i l t e r Supports
1 S t a p l i n g Machine
1 Tray
1 Squeegee
1 Kit
50 Data Sheets
1 Set of I n s t r u c t i o n s
50 P l a s t i c Sample Envelopes
1 Carrying Case
1 Cascade Impactor
50 Coated Aluminum S l i d e s i n F i l e Box
1 Box 1-1/8" Whatman # j l F i l t e r papers
15 Glassene Sample Envelopes
15 Data Sheets
1 Hudson Pump with Rotameter
1 Tripod
87 -
APPENDIX D (Con't)
K - Scintillometer
L = Sleeping Gear
2 Cots, Folding
6 Blankets
P - Dosimeter Kit
- 88 -
APPENDIX E
The procedure for taking and handling each of these samples will be
given in detail so that comparable results may be obtained at all
collecting stations and laboratorieso
- 89 -
&
Precipitation Samples
A
° Collections The sampling trays furnished by NYO have an
area of 9 square feet and are mounted on legs for ease in
setting up. The tray should be erected and a two quart
Mason jar placed under the outlet. In case of heavy rain,,
the jar should be replaced when full, and all jars treated
as one sample»
After all the water has been sucked through the paper, some
drying may be obtained by allowing the aspirator to pull
air through the paper for one or two minutes. The rubber
tubing should then be disconnected at the filter funnel be-
fore turning off the aspirator.
t
Bo Filtration8 This is done exactly as for precipitation sam-
ples s
Collecting stations should send the paper, bag and data sheet
to the specified laboratory, by mail, and if an appreeiabls
saving of time would result, by air mailo
The paper filter is mounted in the head with the rough0 dark
side out toward the entering air« The flow rate and date
and hour of starting should be noted on the data sheets
Since the flow rate may decrease as dust collects, the sams
data must be noted at the end of the runQ
- 91
N.Y. FORM 107
(9-10-511
DATA SHEET
STATION.
CITY JSTATE
TAKEN BY.
Precipitation
Estimated Volume Collected. Dints
Estimated Rainfall. .Inches
Duration, from to.
C Z ) Settled Dust on Tray
i ' Settled Dust on Oummed Paper
I I Airborne Dust
General Remarks
Counting Data:
Results _d/m/sample
_d/m
(unit)
Final Extrapolated Value. .d/m/_
(unit)
Extrapolated to - Date .Hour. .Time Zone.
4«\
• •
COLLECTING S T A T I C I , . . . . . > ( . . . . i o > i < » i . > . i » t i «<»<o Dust on Tr^y !~J L a b o r a t o r y , , . . , . . , . . . . . . . . . . . = . = .«t.<>.<>.»...°o.o.o»«
C i t y . . . . . . . . . . . . . . . . . . . . . . . . S t a t e . . . . . . . . . . . . T i m e Zone,.t. City, «...o•....State..........Time Zone. < , . . . .
Guinned Paper 4 7
Airborne Dust
Start Sample End Sample Rainfall rj_ Rain- Wind Di- Wind First Count at Second Count at Extrap-
Sanple Starting Fxnal
Date Hour Jnoirf all J—f fall rection Velocity Date Hour d/m Date Hour d/mj olated
Number D-ite Hour Rate(cfrn) Rate(cfm)
From To (inches) Value
Remarks
Remarks
Remarks
Remarks
1
Remarks
Remarks
Remarks
'
Remarks
Remarks
Remarks
Remarks
Remarks
APPENDIX G
October 28
Cyclone
Sampler
Sampling Beta Gamma A c t i v i t y % l e s s than
Station Time i n d/min/nP 5 microns
- 9k
91
October 29
Cyclone
Sampler
Sampling Beta G annua A c t i v i t y % l e s s than
Station Time in t d/min /m 5 microns
Cyclone
Sampler
Sampling Beta Gamma Activity
amma Actii % less than
Station Time int d/min/ar 5 microns
Cyclone
Sampler
Sampling Beta Gamma Activity % l e s s than
Station Time in d/mln/m> 5 microns
91
o/
November 1
Cyclone
Sampler
Sampling Beta Gamma A c t i v i t y % l e s s than
Station Time In d/min/n^ 5 microns
Dallas 9 21*00-0200 31 71* 2 0.2
Texas 0200-01*00 0„8 1.5
01*00-0600 108 2*2
0600-0800 5.2 5.7
0800-1000 7.8 5.2
1000-1200 1.3 7.0
1200-11*00 3.5 8.7
ll*CKKL600 9.6 9.6 2,2
1800-2000 52 1*0
1800-2200 60 1*6
2000=21*00 6.9 22
Houston, 21*00-0200 32
Texas l600~l800 9
1800-2000 18
2000-2200 U*
2200-21*00 18
98
November 1
(ConTinTiecI)
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time in d/min/w 5 microns
Omaha, 21*00-0200 L600 5.7 2.7 88
Nebraska 0200-01*00 2»5 h»9 100
0l*00-060Q 5.7 8 100
0600-0800 7.6 5.1 ICO
0800-1000 U.6 93 0
1000-1200 7.0 2.6 3.0 3.7 62
1200-11*00 6.1* 6.8
11*00-1800 7.2 6.8
1800-2200 5.7 9.8
2000-2200 U.6 3.7
Topeka,
Kansas
21*00-0200
21*00-0600
3.0 ha 6.9 2.1*
U*.l*
0200-0600 lo5 7.8 h
060O0800 5.1 3.6 6.6
0800-1000 2.!* 3o3 PoX 5y
1000-1J*00 7.7 2.7 3.9
21*00-1600 33
6.9 ka 98 Cr-
- 99
November 2
Cyclone
Sampler
Sampling Beta Samma A c t i v i t y % l e s s than
Sfa.tion Time i n d/EiixL'nr' 5 microns
—
Corpus C h r i s t i , 180*3-2000 8.6 i*.8 8.6 80
Texas 2000-2200 12 6.9 6»9 62
2200-21*00 7.5 8.6
- 100
November 2
(Continued)
Cyclone
Sampler
Sampler Beta Gamms1 Activity % l e s s than
Station _Time_ in d/min/n^ 5_roicrons
Oklahoma City, 21*00-0200 2*6 1 0*1* 5*2 1*2
Oklahoma 0200-01*00 16 6o5 7.3 111
0]400-0600 6«1 9a 3.0 87
0600-0800 10 9.6 3.0 100
0800-1000 15 22 9.1 77
1000-11*00 32 1**9
11*00-1800 21*
1800-2200 22
2200-21*00 25
101 -
November 3
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time i n d/mln/m?
102
q«j
November 3
(Continue^')
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time in d/min/m3 5 microns
103
November 1*
Cyclone
Sampler
Sampling Beta Gamma A c t i v i t y 2 l e s s than
Station Time 5 miorons
- lol* -
November 1+
(Continued)
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time 5~ microns
-105 -
November
Cyclone
Sampler
Sampling Beta Gamma A kctivity % less than
Station Time m i n d/miaBtAr 5 microns
Dallas, 21*00-0200 17 31
Texas 0200-0J400 1*8 7
OUOO-O6OO 27 3.1+
0800-1000 51 93
0800-1200 100
1000-1600 87 110 51 180
1200-3800 5.1+ 31
1600-2000 1.1 1.6
1800-2200 0.7 0.8
Cyclone
Sampler
Sampling Beta Gamma A c t i v i t y t> less than
Station Time i n d/Wn/m? 5 microns
107
' Jt
November 6
Cyclone
Sampler
Sampling Beta Gamma .Activity % l e s s than
Station Time in L d / m i n / w 5 microns
108 -
November 6
(Continued)
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time in d/min/m? 5 microns
Topeka, 21+00-01*00
Kansas ol+oo-iooo
0800-11+00
Waco, 21*00-0200
Texas 2000-21+00
109 -
. '"M;
November 7
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time in d/min/m? 5 microns
.0<
November 7
(Continued)
Cyclone
Sampler
Sampling Beta Grcumoft A c t i v i t y % less than
Station Time i n d/min/m? 5 microns
- Ill
* '\v
November 8
Cyclone
Sampler
Sampling Beta Gamma Activity % less than
Station Time in "<&/min/ay 5 microns
.
Dallas, 0200-0800 2.3
Texas 0800-1800 1.1
0200-1000 2.8
1000-1800 2.1
./::>
APPENDIX H
d/min./ft.2
(Not Extrapolated)
A B A B
- 113 -
y
APPENDIX H
A B A B
-11U -
APPENDIX H (Cont'd.)
A B A B
31.8 16 hh 72
3-3 3.8 2U 2U
22.3 16.9 236 176
O.U 5.3 88 156
u.u 1.0 16U 88
3.9 0.3 100 96
3.3 5.3 116 176
U.2 3.6 188 1U0
3.U U.8 188 16U
1.7 0.6 988 1176
2.6 0.9 U8 6U
0 0 20 20
0 0 12 16
2.6 2.1 32 20
0 3.5 6U 80
U.6 3.8 16 20
186.8 U50.7 12 2U
0.8 5.6 12 8
262.8 157.2 68 32
82.8 52.1 36 52
21.7 UU.l 56 100
63 .U 3$.9 16 20
3959 27201 16 16
2502.9 31*85.8 52 52
1353.8 863.7 12 20
78.8 161.1 2U 36
218.6 156.2 2U 68
185.7 57.5 80 2U
105.2 11.3 2U 2U
3.7 9.5 16 8
80.5 38 .U 12 12
12 12
8 16
12 8
2U 16
128 28
- 115 -
<
APPENDIX H (Cont'd.)
Station #U6
Mew Cumberland, Pennsylvania
A B
22.6 3U.8
2U.3 28.9
23.2 5.6
19.5 3.3
U.9 18.2
3.7 3.7
0.0 U.3
103.0 86.3
223.U 158.1
U85.8 107.9
220.U 288.2
116 -
f ')
r J. « >