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Article history:
Received 22 July 2009
Received in revised form
5 November 2009
Accepted 21 November 2009
Here I report on the decay processes of microscopic organic residues left on stone tool surfaces after their
use. Residue analysis on ancient stone tools facilitates reconstruction of past activities. This study enables
predictions about the circumstances under which ancient residues preserve. Experimental tool sets with
modern residues were buried for a year in separate deposits at Sterkfontein, Sibudu (South Africa) and
Zelhem (the Netherlands) whose pH and geomorphology varied, they were then analysed using light
microscopy. Biological weathering mainly causes residue decay. In unstable environments rich in
microbes and micro-organisms, residues decay quickly. From an archaeological perspective this means
that sites that are stable, desiccated, waterlogged, extremely acidic or alkaline and extremely cold or hot
sites. Different residue types have different preservation optima and this may lead to a preservation and
perhaps interpretation bias. The preliminary predictive models presented in this paper could aid in the
considered selection of sites and samples.
2009 Elsevier Ltd. All rights reserved.
Keywords:
Residue analysis
Micro-remains
Preservation
Conservation
Decay
Taphonomy
Stone tools
Experimental archaeology
Replication
1. Introduction
It has been argued that researchers are unable to describe the
mechanism of residue decay (Grace, 1996; Odell, 2001). This paper
aims to investigate some of these taphonomic issues. Grace
observes that residue analysts . simply record a phenomenon
(.) and then make functional interpretations by analogy without
having explained the process that gave rise to the phenomenon.
(Grace, 1996, 214). Odell argues that residue analysts are inclined
to consider what they see, not what is missing (Odell, 2001, 63).
Although these issues are acknowledged and in some cases
examined (e.g. Barton, 2009; Barton et al., 1998; Fullagar, 1988,
1998; Haslam, 2004; Jones, 2009; Lombard and Wadley, 2007; Lu,
2006; Rots and Williamson, 2004; Wadley and Lombard, 2007),
they remain essentially unresolved. Potentially the results from
residue studies may be oversimplied, or worse inaccurate.
Stone tool micro-residue analysis aims to identify microscopic
remains or traces that are left on a tools surface after use. Analysts
have identied organic plant and animal remains and inorganic
deposits. Residue analysis is generally conducted with a direct or
indirect light microscope, using a range of magnications (between
50 and 800 times), an experimental comparative collection and
sometimes an ethno-archaeological comparative collection
(Anderson, 1980; Bruier, 1976; Fullagar et al., 1996, 1999; Loy, 1997;
Miller, 1979; Rots and Williamson, 2004; Williamson, 2000a,b).
The identication of processed materials is of relevance to
a wide range of research questions (Bruier, 1976; DominguezRodrigo et al., 2001; Fullagar, 2006; Fullagar and Jones, 2004; Hardy
et al., 2008; Horrocks et al., 2007; Hurst et al., 2002; Lombard,
2005; Piperno et al., 2004; Staller and Thompson, 2002). Residues
themselves may also serve as a source for further investigation, for
example DNA analysis (e.g. Hardy et al., 1997; Nelson et al., 1986;
Williamson, 2000b) and they can be used to study rare artefacts for
additional information (e.g. Barton, 2007; Loy, 1998; Loy and Dixon,
1998).
As yet, it is unclear to which extent residues on tools are the
result of use or of taphonomic processes. As residues are expected
to be inuenced by taphonomy, direct analogies between use and
remains are problematic (Grace, 1996; Haslam, 2006; Odell, 2001),
especially when quantitative spatial analyses are not conducted on
representative samples (e.g. Lombard, 2005, 2007; Wadley and
Lombard, 2007). When analysts are able to describe the mechanism
of residue preservation and predict under which circumstances
(what) residues preserve, residue analysis has great potential.
There have been many investigations into the molecular decay
of blood and fat (e.g. Cattaneo et al., 1993, 1991; Eisele et al., 1995;
Evershed, 2008; Evershed et al., 2001; Evershed and Tuross, 1996;
Gurnkel and Franklin, 1988; Kooyman et al., 1992; Tuross et al.,
1996). The decay and taphonomy of blood and starch has been
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