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Research Article
Nuclear Track Detection of Radon Activities among Branded
Bottled Water and Locally Bottled Water in Afghanistan
Marufat Fazli
Lecturer, Department of Physics Education Faculty, Jawzjan University, Sheberghan, Afghanistan
Email: marufatfazli01@gmail.com
In this study, radon activities and exhalation rate were calculated in ten bottled waters (branded
and locally). The measurements were performed by nuclear track detectors. The findings of the
study indicated that radon activities in all the analysed samples of branded bottled waters were
found to be lower than the maximum contamination level recommended for drinking water by
United State Public Health Service (USEPA) and World Health Organization (WHO) guidelines
value. Further, the result showed that the mean value of radon activity in local bottled waters is
higher than the mean value from branded bottled waters. The results revealed that revealed that
all investigated samples of branded bottled water are safe for consumption in Afghanistan from
the point of radon activity.
Keywords: Radon activity, bottled water, radon emission, radioactivity.
INTRODUCTION
Water is the most important source for life and makes up sex, nutritional characteristics, lifestyle, and health status
70 - 75% of total body weight. While 70% of the world's (USPHS and USEPA, 1990).
surface is covered by water, only 0.3 % of the total water
resources on earth is drinkable and suitable for daily use. Radon is a naturally occurring radioactive element. It is a
Human race provides their water from surface water and colourless, odourless and chemically inert gas and has no
ground water. Ground water is more radioactive than taste. It can only be measured with special equipment.
surface water since it passes through rock and soil Radon is also fairly soluble in water and organic solvents.
formations, dissolves many compounds, minerals and Although reaction with other compounds is comparatively
radioactive substances. The radionuclides in drinking rare, it is not completely inert and forms stable molecules
water are members of three natural radioactive series. with highly electronegative ions. The radioactive decay of
These are the uranium series, the thorium series and the radon produces floating subatomic particles that can
actinium series. The specific elements of concern are damage living cells. When radon is inhaled, 30% of the
radium, radon and uranium. The nuclides of the uranium radon progeny comes in to contact with air passage in the
series which can be dangerous to health because of their lung and adhere to the surfaces. The ingestion of radon
presence in drinking water are 226Ra and 222Rn. and radium from water can give rise to an additional
exposure dose to the stomach and whole body.
The 226Ra (half-life 1622 years) decays to 222Rn by emitting
alpha particles. Thereafter, 222Rn undergoes multiple The measurement of radioactivity in drinking water permits
alpha and beta decays in succession resulting in various us to determine the exposure of the population to radiation
isotopes of polonium, astatine, bismuth, thallium, and lead from the habitual consumption of water (Duenas et al.,
(Eisenbud and Gesell, 1997). Making the analysis of 1999). The radionuclides in drinking water are members of
exposure to a substance such as radium, several factors three natural radioactive series. These are the uranium
determine which effects may occur and also the severity of series, the thorium series and the actinium series. The
these effects. Among those factors are the dose, the specific elements of concern are radium (Ra), radon (Rn)
duration of exposure, the manner of exposure (inhalation, and uranium (U). The nuclides in the uranium series that
ingestion or contact), other agents to which the individual may pose a health risk because of their presence in
is exposed as well as individual characteristics like an age, drinking water are 238U, 226Ra and 222Rn.
Nuclear Track Detection of Radon Activities among Branded Bottled Water and Locally Bottled Water in Afghanistan
Fazli M. 098
226Ra is considered because, apart from being an emitter where ρ is the track density on the detector, T is the
of alpha radiation, it has a chemical behaviour with exposure time and η is the calibration factor (tracks cm-2
alkaline-earth characteristics similar to that of calcium. recorded per Bq m-3h-1).
This chemical behaviour produces a tendency to be
concentrated in bones resulting in irradiation of bone The radon activity in water, Rnwater, was calculated by
marrow. using a model proposed by Al-Bataina et al., (1997):
Rnwater = (λ RnAir h T)/L ……………………………. (2)
MATERIALS AND METHODS where λ is the radon decay constant, h is the distance from
surface of water in sample cup to detector, T is the
Five samples each of bottled water from various brand exposure time and L is depth of the sample.
names (BB) and locally bottled water (LB) were collected The radon exhalation rates, Ewater, were calculated using
from the local market. For measurements purpose, 150 ml the following equation (Baykara et al., 2006; Alshahri,
was collected for each sample tested. Branded water 2014):
bottles were purchased from various places of Ewater (mBq m-2 h-1) = (ρV λ /A)/ η Teff ………………. (3)
Afghanistan.
where ρ is the track density measured in the CR-39
Radon Monitoring System detector (track cm-2), V is effective volume of detection
chamber (150 cm3), λ is the radon decay constant, η is the
The radon monitoring system consists of two tightly calibration factor (tracks cm-2 recorded per Bq m-3 h-1), A is
coupled cup-type plastic containers (Kadi and Al-Eryani, the surface area of the sample (m2) and Teff is the effective
2012). One of them is a detection chamber and the other exposure time which is defined as:
is a water container. Solid-state nuclear track detectors
CR-39, 2.5 × 2.5 cm in size, were attached to the bottom Teff = T – (1/ λ) (1 – e- λ T) ……………………………. (4)
of detection chamber in an empty volume of 150 ml. The
water container had approximately 150 ml water. There is
a round hole (D = 1.5 cm) in the middle of the lid of the RESULTS AND DISCUSSION
detection chamber, which is covered with a sponge filter.
The function of this filter is to reduce the humidity in the 222RnAir (Bq m-3) activity was determined in the range of
detection chamber and to discriminate against thoron 6.87 and 11.0 in the case of local bottled water. The values
220Rn (half-life is 55.6 s) by hindering its diffusion into the were between 2.04 and 4.11 for branded bottled water
volume of the detection. The two coupled cup-type (Fig-1). Similarly, the values of 222Rnwater (Bq m-3) were
containers were stored for more than one month to allow higher in local bottled water than branded bottled water
radioactive equilibrium to be reached in all samples. (Fig-2). EA (mBq m-2 h-1) were in the range of 0.59 and
4.81 which was again higher in local bottled water (Fig-3).
Etching and Scanning System By comparing the radon activity in bottled water from
various sources, the mean value of radon activity in non-
After exposure to radon, the detectors were collected from branded bottled water is higher than mean values in
the detection chambers and etched by using 6.25 M NaOH branded bottled water. This is probably due to most of local
solution (250 grams of solid NaOH made up to one liter of non-branded bottled water were produced from ground
water) at 70°C in a water bath for 6 hours. After etching, well water which contain activity of higher radon.
the detectors were removed from the solution and cleaned
in distilled water for 15 s, then, transferred to a 2%
neutralizing solution (by adding 2 parts glacial acetic acid
to 98 parts distilled water) for 30 min. Finally, the detectors
were removed from the neutralizing solution and placed in
distilled water for 10 min then placed in a drying cabinet for
20 minutes.
Theoretical Calculations
Nuclear Track Detection of Radon Activities among Branded Bottled Water and Locally Bottled Water in Afghanistan
J. Phys. Astron. Res. 099
REFERENCES
CONCLUSION
Nuclear Track Detection of Radon Activities among Branded Bottled Water and Locally Bottled Water in Afghanistan